Manipulating the metal-to-insulator transition and magnetic properties in manganite thin films via epitaxial strain

نویسندگان

چکیده

Strain engineering of epitaxial transition metal oxide heterostructures offers an intriguing opportunity to control electronic structures by modifying the interplay between spin, charge, orbital, and lattice degrees freedom. Here, we demonstrate that structure, magnetic transport properties ${\mathrm{La}}_{0.9}{\mathrm{Ba}}_{0.1}{\mathrm{MnO}}_{3}$ thin films can be effectively controlled strain. Spectroscopic studies first-principles calculations reveal orbital occupancy in Mn ${e}_{g}$ orbitals switched from ${d}_{3{z}^{2}\ensuremath{-}{r}^{2}}$ ${d}_{{x}^{2}\ensuremath{-}{y}^{2}}$ varying strain compressive tensile. The change associated with $3d$-O $2p$ hybridization leads dramatic modulation strained films. Under moderate tensile strain, emergent ferromagnetic insulating state enhanced Curie temperature 215 K is achieved. These findings not only deepen our understanding structures, system, but also use as effective knob tune related physical for potential spintronic device applications.

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ژورنال

عنوان ژورنال: Physical review

سال: 2022

ISSN: ['0556-2813', '1538-4497', '1089-490X']

DOI: https://doi.org/10.1103/physrevb.105.165426